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63) that an uninterestingly restrictive condition for atmospheric calculations. (ii) Rapid collisions. At high pressures, the collisional rate is high, the 40 ATMOSPHERIC RADIATION vibrational relaxation time is short, and r)/

We define and We can now make a variety of choices for the Stokes parameters: (Iv, Qv, Uv, Vv) is one possibility; (/<°, /tr), f/ v , V r ) is another. Four parameters are more than are necessary to specify an elliptically 26 ATMOSPHERIC RADIATION polarized beam, for which the following relation exists, A more general field may contain many independent, polarized components. 28) no longer holds. Then all four parameters are required to define the field. Natural (or unpolarized) light has /1° = /lr), and therefore Qv = Uv = Vv = 0.

Wofsy, S. , and McElroy, M. , 1978, "Atmospheric chemistry: Response to human influence," Phil. Trans. Roy. Soc. London Ser. A 290, 187. The Hawaiian carbon dioxide measurements are reported by Bacastow, R. , Keeling, C. , and Whorf, T. , 1985, "Seasonal amplitude increase in the atmospheric CO2 concentration at Mauna Loa, Hawaii, 19591982," J. Geophys. Res. 90, 10529. Isotopic ratios are given by Evans, R. , 1955, The atomic nucleus. New York: McGraw-Hill. Data on atmospheric aerosol and clouds are reviewed by Mason, B.

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